We show that to understand harmonic generation from molecules undergoing a large change in configuration, multiple ionization continua must be considered. After exciting large amplitude vibrations in an N2O4 dimer, bright bursts of harmonics are emitted at the outer turning point of the vibration.
BT - Ultrafast Phenomena XVI CY - Berlin, Heidelberg DA - 2009-01 DO - 10.1007/978-3-540-95946-5_21 N2 -We show that to understand harmonic generation from molecules undergoing a large change in configuration, multiple ionization continua must be considered. After exciting large amplitude vibrations in an N2O4 dimer, bright bursts of harmonics are emitted at the outer turning point of the vibration.
PB - Springer Berlin Heidelberg PP - Berlin, Heidelberg PY - 2009 SN - 978-3-540-95946-5 SP - 63 EP - 65 T2 - Ultrafast Phenomena XVI TI - Probing Dynamics in Polyatomic Molecules Using High Harmonic Generation: the Role of Ionization Continua ER -