TY - JOUR KW - General Physics and Astronomy AU - Colin Kennedy AU - Eric Oelker AU - John Robinson AU - Tobias Bothwell AU - Dhruv Kedar AU - William Milner AU - Edward Marti AU - Andrei Derevianko AU - Jun Ye AB - We conduct frequency comparisons between a state-of-the-art strontium optical lattice clock, a cryogenic crystalline silicon cavity, and a hydrogen maser to set new bounds on the coupling of ultralight dark matter to standard model particles and fields in the mass range of 10−16 − 10−21eV. The key advantage of this two-part ratio comparison is the differential sensitivity to time variation of both the fine-structure constant and the electron mass, achieving a substantially improved limit on the moduli of ultralight dark matter, particularly at higher masses than typical atomic spectroscopic results. Furthermore, we demonstrate an extension of the search range to even higher masses by use of dynamical decoupling techniques. These results highlight the importance of using the best-performing atomic clocks for fundamental physics applications, as all-optical timescales are increasingly integrated with, and will eventually supplant, existing microwave timescales. BT - Physical Review Letters DA - 2020-11 DO - 10.1103/physrevlett.125.201302 IS - 20 N2 - We conduct frequency comparisons between a state-of-the-art strontium optical lattice clock, a cryogenic crystalline silicon cavity, and a hydrogen maser to set new bounds on the coupling of ultralight dark matter to standard model particles and fields in the mass range of 10−16 − 10−21eV. The key advantage of this two-part ratio comparison is the differential sensitivity to time variation of both the fine-structure constant and the electron mass, achieving a substantially improved limit on the moduli of ultralight dark matter, particularly at higher masses than typical atomic spectroscopic results. Furthermore, we demonstrate an extension of the search range to even higher masses by use of dynamical decoupling techniques. These results highlight the importance of using the best-performing atomic clocks for fundamental physics applications, as all-optical timescales are increasingly integrated with, and will eventually supplant, existing microwave timescales. PB - American Physical Society (APS) PY - 2020 SE - 201302 EP - 201302 T2 - Physical Review Letters TI - Precision Metrology Meets Cosmology: Improved Constraints on Ultralight Dark Matter from Atom-Cavity Frequency Comparisons UR - https://link.aps.org/doi/10.1103/PhysRevLett.125.201302 VL - 125 SN - 0031-9007, 1079-7114 ER -